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Vibration and two-photon absorption

The rigorous and transparent treatment of the effects of nuclear vibrational motion in two-photon absorption (TPA) was discussed. Perturbation formula for diatomic molecules were developed and applied to the X¹Σ+–A¹Π transition in CO. The analysis showed that the vibrations played an important role in TPA, just as their role in the calculation of conventional nonlinear optical (NLO) hyperpolarizabilities

© Journal of Chemical Physics, 2002, vol. 116, núm. 22, p. 9729-9739

American Institute of Physics

Author: Bishop, David M.
Luis Luis, Josep Maria
Kirtman, Bernard
Date: 2002
Abstract: The rigorous and transparent treatment of the effects of nuclear vibrational motion in two-photon absorption (TPA) was discussed. Perturbation formula for diatomic molecules were developed and applied to the X¹Σ+–A¹Π transition in CO. The analysis showed that the vibrations played an important role in TPA, just as their role in the calculation of conventional nonlinear optical (NLO) hyperpolarizabilities
Format: application/pdf
Citation: Bishop, David M., Luis, Josep Maria, i Kirtman, Bernard (2002). Vibration and two-photon absorption. Journal of Chemical Physics, 116 (22), 9729-9739. Recuperat 23 desembre 2010, a http://link.aip.org/link/JCPSA6/v116/i22/p9729/s1
ISSN: 0021-9606 (versió paper)
1089-7690 (versió electrònica)
Document access: http://hdl.handle.net/10256/3193
Language: eng
Publisher: American Institute of Physics
Collection: Reproducció digital del document publicat a: http://dx.doi.org/10.1063/1.1477179
Articles publicats (D-Q)
Is part of: © Journal of Chemical Physics, 2002, vol. 116, núm. 22, p. 9729-9739
Rights: Tots els drets reservats
Subject: Absorció de la llum
Col·lisions (Física nuclear)
Fotons
Collisions (Nuclear physics)
Light absorption
Photons
Title: Vibration and two-photon absorption
Type: info:eu-repo/semantics/article
Repository: DUGiDocs

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